As the additive manufacturing process gains worldwide importance, the need for bio-based materials, especially for in-home polymeric use, also increases. This work aims to develop a composite of polylactic acid (PLA) and nanofibrillated cellulose (NFC) as a sustainable approach to reinforce the currently commercially available PLA. The studied materials were composites with 5 and 10% NFC that were blended and extruded. Mechanical, structural, and thermal characterization was made before its use for 3D printing. It was found that the inclusion of 10% NFC increased the modulus of elasticity in the filaments from 2.92 to 3.36 GPa. However, a small decrease in tensile strength was observed from 55.7 to 50.8 MPa, which was possibly due to the formation of NFC aggregates in the matrix. This work shows the potential of using PLA mixed with NFC for additive manufacturing.